Search results for "Materials Science | Hot Paper"
showing 10 items of 1457 documents
Topological transition in Pb1-xSnxSe using Meta-GGA
2023
We calculate the mirror Chern number (MCN) and the band gap for the alloy Pb1-xSnxSe as a function of the concentration x by using virtual crystalline approximation. We use the electronic structure from the relativistic density functional theory calculations in the Generalized-Gradient- Approximation (GGA) and meta-GGA approximation. Using the modified Becke-Johnson meta- GGA functional, our results are comparable with the available experimental data for the MCN as well as for the band gap. We advise to use modified Becke-Johnson approximation with the parameter c=1.10 to describe the transition from trivial to topological phase for this class of compounds.
Role of precursor composition in the polymorph transformations, morphology control and ferromagnetic properties of nanosized TiO$_2$
2021
Pure phase and mixed phase TiO$_2$ nanoparticles have been produced using a pyrolytic method from a non-aqueous carboxylate precursor. The precursor was prepared by a multiphase cation exchange using pentanoic acid (C$_4$H$_9$COOH). The thermal stability, polymorph content, morphology, size distribution and surface region of the produced nanoparticles were studied by TGA/DSC, XRD, FTIR and TEM. High quality monodisperse nanoparticles have been produced in the size range from 7 to 27 nm. The nanoparticles showed room temperature ferromagnetism revealed by VSM within bound polaron model. The carboxylate precursor is a good alternative to standard sol-gel to produce nanoparticles free from imp…
Ultrafast laser-induced spin-lattice dynamics in the van der Waals antiferromagnet CoPS3
2023
CoPS3 stands out in the family of the van der Waals antiferromagnets XPS3 (X=Mn, Ni, Fe, Co) due to the unquenched orbital momentum of the magnetic Co2+ ions which is known to facilitate the coupling of spins to both electromagnetic waves and lattice vibrations. Here, using a time-resolved magneto-optical pump-probe technique we experimentally study the ultrafast laser-induced dynamics of mutually correlated spins and lattice. It is shown that a femtosecond laser pulse acts as an ultrafast heater and thus results in the melting of the antiferromagnetic order. At the same time, the resonant pumping of the 4T1g - 4T2g electronic transition in Co2+ ions effectively changes their orbital moment…
Dielectric properties of PLZT-x/65/35 (2 \leqslant x \leqslant 13) under mechanical stress, electric field and temperature loading
2013
We investigated the effect of uniaxial pressure (0-1000 bars) applied parallely to the ac electric field on dielectric properties of PLZT-x/65/35 (2 \leqslant x \leqslant 13) ceramics. There was revealed a significant effect of the external stress on these properties. The application of uniaxial pressure leads to the change of the peak intensity of the electric permittivity (\varepsilon), of the frequency dispersion as well as of the dielectric hysteresis. The peak intensity $\varepsilon$ becomes diffused/sharpened and shifts to a higher/lower temperatures with increasing the pressure. It was concluded that the application of uniaxial pressure induces similar effects as increasing the Ti io…
Application of relative configurational entropy as a measure of spatial inhomogeneity to Co/C film evolving along the temperature
2001
Based on the digitized electron micrographs, we investigate a temperature evolution of Co/C film. The simple in usage quantitative characterization of the spatial disorder for systems of point objects has been employed. We show that a dominant increase of spatial inhomogeneity of cobalt phase is shifted towards the larger length scales along the sample heating temperature. The results allow the subtle differences of spatial inhomogeneity in thin metallic films to be explored.
Unified topological characterization of electronic states in spin textures from noncommutative K-theory
2021
The nontrivial topology of spin systems such as skyrmions in real space can promote complex electronic states. Here, we provide a general viewpoint at the emergence of topological electronic states in spin systems based on the methods of noncommutative K-theory. By realizing that the structure of the observable algebra of spin textures is determined by the algebraic properties of the noncommutative hypertorus, we arrive at a unified understanding of topological electronic states which we predict to arise in various noncollinear setups. The power of our approach lies in an ability to categorize emergent topological states algebraically without referring to smooth real- or reciprocal-space qu…
Interfacial Oxide Modulated unique Exchange Bias in CrPS4/Fe3GeTe2 van der Waals heterostructures
2023
Two-dimensional van der Waals heterostructures are an attractive platform for studying exchange bias due to their defect free and atomically flat interfaces. Chromium thiophosphate (CrPS4), an antiferromagnet, has uncompensated magnetic spins in a single layer that make it an excellent candidate for studying exchange bias. In this study, we examined the exchange bias in CrPS4/Fe3GeTe2 van der Waals heterostructures using anomalous Hall measurements. Our results show that the exchange bias strength is robust for clean interfaces, with a hysteresis loop shift of about 55 mT at 5 K for few-layer Fe3GeTe2, which is larger than that obtained in most van der Waals AFM/FM heterostructures. However…
Strain hardening-softening oscillations induced by nanoindentation in bulk solids
2016
Nanoindentation is a widely used method for sensitive exploration of the mechanical properties of micromechanical systems. We derived an empirical analysis technique to extract stress-strain field gradient and divergence representations from nanoindentation measurements. With this approach local gradients and heterogeneities can be discovered to obtain more detail about the sample's microstructure, thus enhancing the analytic capacity of the nanoindentation technique. We analysed nanoindentation tests of bulk solid substrates, namely bearing and tooling steel, and fused silica. Oscillations of the stress-strain field gradient and divergence induced in the subsurface layer by the nanoindenta…
Engineering the molecular structure to optimize the spin Hall signal in organics
2020
In this study, by engineering the molecular structure, we optimize the spin Hall conductivity and the spin Hall angle in organics by more than five and three orders of magnitude, respectively. We identify two important characteristics of organic molecules, namely substitution of heavy elements and the torsion angles between constituent units of the polymer, which have significant effects on the spin Hall signal. These characteristics are directly related to the spin-orbit coupling and the energetic disorder, both of which offer a wide scope of chemical tunability in high-mobility polymers. We compute the spin Hall characteristics for easily synthesized molecules and identify candidates to e…
Enhanced thermally-activated skyrmion diffusion in synthetic antiferromagnetic systems with tunable effective topological charge
2022
Magnetic skyrmions, topologically-stabilized spin textures that emerge in particular magnetic systems, have attracted attention due to a variety of electromagnetic responses that are governed by the topology. A well-studied effect of topology on the deterministic and drift motion under a nonequilibrium excitation is the so-called skyrmion Hall effect. For stochastic diffusive motion, the effect of topology is expected to have a drastically stronger impact, but the predicted even qualitative impact has not been demonstrated. The required tuning of the topology to achieve zero effective topological charge can be achieved using antiferromagnetic skyrmions. However, the diffusive motion has pre…